| Basil in The Silver Chalice |
| Capt. Edward W. Hall, Jr. in The Rack |
| Rocky in Somebody Up There Likes Me |
| Larry Maddux in The Helen Morgan Story |
| Capt. Jack Harding in Until They Sail |
| Brick Pollitt in Cat on a Hot Tin Roof |
| Billy The Kid in The Left Handed Gun |
| Ben Quick in The Long, Hot Summer |
| Harry Bannerman in Rally 'Round the Flag, Boys! |
| Anthony Judson Lawrence in The Young Philadelphians |
| Ari Ben Canaan in Exodus |
| David Alfred Eaton in From the Terrace |
| Eddie Felson in The Hustler |
| Ram Bowen in Paris Blues |
| Chance Wayne in Sweet Bird of Youth |
| Hud Bannon in Hud |
| Steve Sherman in A New Kind of Love |
| Andrew Craig in The Prize |
| Juan Carrasco in The Outrage |
| Larry Flint in What a Way to Go! |
| Armand Denis in Lady L |
| Lew Harper in Harper |
| Prof. Michael Armstrong in Torn Curtain |
| Luke in Cool Hand Luke |
| John Russell in Hombre |
| Harry Frigg in The Secret War of Harry Frigg |
| Butch Cassidy in Butch Cassidy and the Sundance Kid |
| Capua in Winning |
| Self and narrated by in The Making of 'Butch Cassidy and the Sundance Kid' |
| Rheinhardt in WUSA |
| Hank in Sometimes a Great Notion |
| Judge Roy Bean in The Life and Times of Judge Roy Bean |
| Jim Kane in Pocket Money |
| Rearden in The MacKintosh Man |
| Henry Gondorff in The Sting |
| Doug Roberts in The Towering Inferno |
| Lew Harper in The Drowning Pool |
| William F. Cody in Buffalo Bill and the Indians, or Sitting Bull's History Lesson |
| Reggie in Slap Shot |
| Essex in Quintet |
| Hank Anderson in When Time Ran Out... |
| Michael Colin Gallagher in Absence of Malice |
| Murphy in Fort Apache the Bronx |
| Frank Galvin in The Verdict |
| Harry Keach in Harry & Son |
| Eddie in The Color of Money |
| Earl Long in Blaze |
| General Leslie R. Groves in Fat Man and Little Boy |
| Walter Bridge in Mr. & Mrs. Bridge |
| Sidney J. Mussburger in The Hudsucker Proxy |
| Sully in Nobody's Fool |
| Harry Ross in Twilight |
| Dodge in Message in a Bottle |
| Henry in Where the Money Is |
| Doc Hudson in Cars |
| Teller in The Meerkats |
| Narrator in The Price of Sugar |