| Wade Lewis in Inside Daisy Clover |
| Captain Hank Wilson in Situation Hopeless -- But Not Serious |
| Bubber Reeves in The Chase |
| Owen in This Property Is Condemned |
| Paul Bratter in Barefoot in the Park |
| The Sundance Kid in Butch Cassidy and the Sundance Kid |
| Chappellet in Downhill Racer |
| Cooper in Tell Them Willie Boy Is Here |
| Halsy Knox in Little Fauss and Big Halsy |
| Self and narrated by in The Making of 'Butch Cassidy and the Sundance Kid' |
| Bill McKay in The Candidate |
| Dortmunder in The Hot Rock |
| Jeremiah Johnson in Jeremiah Johnson |
| Johnny Hooker in The Sting |
| Hubbell Gardiner in The Way We Were |
| Narrator in Broken Treaty at Battle Mountain |
| Jay Gatsby in The Great Gatsby |
| Waldo Pepper in The Great Waldo Pepper |
| Turner in Three Days of the Condor |
| Bob Woodward in All the President's Men |
| Sonny in The Electric Horseman |
| Henry Brubaker in Brubaker |
| Roy Hobbs in The Natural |
| Denys in Out of Africa |
| Tom Logan in Legal Eagles |
| Narrator in Changing Steps |
| Narrator in To Protect Mother Earth |
| Narrator in Yosemite: The Fate of Heaven |
| Jack Weil in Havana |
| Narrator in Incident at Oglala |
| Bishop in Sneakers |
| John Gage in Indecent Proposal |
| Warren Justice in Up Close & Personal |
| Tom Booker in The Horse Whisperer |
| Narrator in Following the Tundra Wolf |
| Nathan Muir in Spy Game |
| General Irwin in The Last Castle |
| Wayne Hayes in The Clearing |
| Einar Gilkyson in An Unfinished Life |
| Professor Stephen Malley in Lions for Lambs |
| Bill Bryson in A Walk in the Woods |
| Jim Grant in The Company You Keep |
| Narrator in A Fierce Green Fire: The Battle for A Living Planet |
| Alexander Pierce in Captain America: The Winter Soldier |
| Our Man in All Is Lost |
| Meacham in Pete's Dragon |
| Forrest Tucker in The Old Man & the Gun |
| Dan Rather in Truth |
| Louis Waters in Our Souls at Night |
| Thomas in The Discovery |
| Narrator in Out of the Many, the One |
| Narrator in The Big Bang |
| Narrator in Earth: One Amazing Day |
| Narrator in Buttons, A New Musical Film |
| Lewis Wade in Inside Daisy Clover |
| Nick Sloan in The Company You Keep |